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Fundamental studies of Triply Vibrat...

The University of Wisconsin - Madison.

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Fundamental studies of Triply Vibrationally Enhanced Four-Wave Mixing spectroscopy.

Record Type:	Electronic resources : Monograph/item
Title/Author:	Fundamental studies of Triply Vibrationally Enhanced Four-Wave Mixing spectroscopy./
Author:	Rickard, Mark Alan.
Description:	166 p.
Notes:	Adviser: John C. Wright.
Contained By:	Dissertation Abstracts International69-05B.
Subject:	Chemistry, Analytical. -
Online resource:	http://pqdd.sinica.edu.tw/twdaoapp/servlet/advanced?query=3314288
ISBN:	9780549633594

Fundamental studies of Triply Vibrationally Enhanced Four-Wave Mixing spectroscopy.
Rickard, Mark Alan.

Fundamental studies of Triply Vibrationally Enhanced Four-Wave Mixing spectroscopy. - 166 p.

Adviser: John C. Wright.

Thesis (Ph.D.)--The University of Wisconsin - Madison, 2008.

Triply Vibrationally Enhanced Four-Wave Mixing (TRIVE FWM) is a coherent multidimensional spectroscopy that provides significant structural and dynamical information about molecules. It utilizes three mid-infrared laser beams to probe coherences between vibrational states. Continued development of TRIVE FWM involves understanding specific features, such as quantum beating and coherence transfer, and extending its application to common types of organic molecules. Frequency-domain quantum beating appears as a spectral line-splitting that oscillates as a function of the time delay between the laser pulses. The observed quantum beating in nickel(0) triphenylphosphine tricarbonyl defined the frequency difference between two unresolved vibrational states. TRIVE FWM experiments investigated coherence transfer, an amplitude-level process in which a coherence evolves to a different coherence without loss of phase information, in nickel(0) bis(triphenylphosphine) dicarbonyl and rhodium(I) dicarbonyl acetylacetonate. TRIVE FWM can isolate coherence transfer processes and resolve the coherence pathways that are responsible for coherence transfer. Finally, TRIVE FWM experiments examined the interactions of ring stretching modes in pyridine, quinoline, and 1,3-dichlorobenzne and C--H bending and stretching modes in octane and dotriacontane. The experiments provide new insights into important interactions between these vibrational modes in aromatic and alkane molecules.

ISBN: 9780549633594Subjects--Topical Terms:

586156
Chemistry, Analytical.

Fundamental studies of Triply Vibrationally Enhanced Four-Wave Mixing spectroscopy.
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020 $a 9780549633594
035 $a (UMI)AAI3314288
035 $a AAI3314288
040 $a UMI $c UMI
100 1 $a Rickard, Mark Alan. $3 1030673
245 1 0 $a Fundamental studies of Triply Vibrationally Enhanced Four-Wave Mixing spectroscopy.
300 $a 166 p.
500 $a Adviser: John C. Wright.
500 $a Source: Dissertation Abstracts International, Volume: 69-05, Section: B, page: 2967.
502 $a Thesis (Ph.D.)--The University of Wisconsin - Madison, 2008.
520 $a Triply Vibrationally Enhanced Four-Wave Mixing (TRIVE FWM) is a coherent multidimensional spectroscopy that provides significant structural and dynamical information about molecules. It utilizes three mid-infrared laser beams to probe coherences between vibrational states. Continued development of TRIVE FWM involves understanding specific features, such as quantum beating and coherence transfer, and extending its application to common types of organic molecules. Frequency-domain quantum beating appears as a spectral line-splitting that oscillates as a function of the time delay between the laser pulses. The observed quantum beating in nickel(0) triphenylphosphine tricarbonyl defined the frequency difference between two unresolved vibrational states. TRIVE FWM experiments investigated coherence transfer, an amplitude-level process in which a coherence evolves to a different coherence without loss of phase information, in nickel(0) bis(triphenylphosphine) dicarbonyl and rhodium(I) dicarbonyl acetylacetonate. TRIVE FWM can isolate coherence transfer processes and resolve the coherence pathways that are responsible for coherence transfer. Finally, TRIVE FWM experiments examined the interactions of ring stretching modes in pyridine, quinoline, and 1,3-dichlorobenzne and C--H bending and stretching modes in octane and dotriacontane. The experiments provide new insights into important interactions between these vibrational modes in aromatic and alkane molecules.
590 $a School code: 0262.
650 4 $a Chemistry, Analytical. $3 586156
650 4 $a Chemistry, Physical. $3 560527
690 $a 0486
690 $a 0494
710 2 $a The University of Wisconsin - Madison. $3 626640
773 0 $t Dissertation Abstracts International $g 69-05B.
790 $a 0262
790 1 0 $a Wright, John C., $e advisor
791 $a Ph.D.
792 $a 2008
856 4 0 $u http://pqdd.sinica.edu.tw/twdaoapp/servlet/advanced?query=3314288