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Investigation of Sulfide-based Solid...

Kompella, Christopher,

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Investigation of Sulfide-based Solid Electrolytes for Sodium All-Solid-State Rechargeable Batteries /

Record Type:	Electronic resources : Monograph/item
Title/Author:	Investigation of Sulfide-based Solid Electrolytes for Sodium All-Solid-State Rechargeable Batteries // Christopher Kompella.
Author:	Kompella, Christopher,
Description:	1 electronic resource (63 pages)
Notes:	Source: Masters Abstracts International, Volume: 78-11.
Contained By:	Masters Abstracts International78-11.
Subject:	Nanoscience. -
Online resource:	https://pqdd.sinica.edu.tw/twdaoapp/servlet/advanced?query=10260155
ISBN:	9781369696837

Investigation of Sulfide-based Solid Electrolytes for Sodium All-Solid-State Rechargeable Batteries /
Kompella, Christopher,

Investigation of Sulfide-based Solid Electrolytes for Sodium All-Solid-State Rechargeable Batteries /Christopher Kompella. - 1 electronic resource (63 pages)

Source: Masters Abstracts International, Volume: 78-11.

All-solid-state sodium-ion batteries are promising candidates for large-scale energy storage applications. The key enabler for an all-solid-state architecture is a sodium solid electrolyte that exhibits high Na+ conductivity at ambient temperatures, as well as excellent phase and electrochemical stability. In this work, we present the synthesis of a novel Cl-doped tetragonal Na 3PS4 (t-Na3−xPS4−xCl x) solid electrolyte with a room-temperature Na+ conductivity exceeding 1 mS cm−1. We demonstrate that an all-solid-state TiS2/ t-Na3−xPS4−xClx/Na cell utilizing this solid electrolyte can be cycled at room-temperature at a rate of C/10 with a capacity of over 100 mAh g−1 over 10 cycles. Finally, we provide experimental evidence that this excellent electrochemical performance is not only due to the high Na+ conductivity of the solid electrolyte, but also due to the effect that "salting" Na3PS4 has on the formation of an electronically insulating, ionically conducting solid electrolyte interphase.

English

ISBN: 9781369696837Subjects--Topical Terms:

587832
Nanoscience.
Subjects--Index Terms:

Battery

Investigation of Sulfide-based Solid Electrolytes for Sodium All-Solid-State Rechargeable Batteries /
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100 1 $a Kompella, Christopher, $e author. $3 3816037
245 1 0 $a Investigation of Sulfide-based Solid Electrolytes for Sodium All-Solid-State Rechargeable Batteries / $c Christopher Kompella.
264 1 $a Ann Arbor : $b ProQuest Dissertations & Theses, $c 2017
300 $a 1 electronic resource (63 pages)
336 $a text $b txt $2 rdacontent
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500 $a Source: Masters Abstracts International, Volume: 78-11.
500 $a Publisher info.: Dissertation/Thesis.
500 $a Advisors: Meng, Ying Shirley Committee members: Luo, Jian; Ong, Shyue Ping.
502 $b M.S. $c University of California, San Diego $d 2017.
520 $a All-solid-state sodium-ion batteries are promising candidates for large-scale energy storage applications. The key enabler for an all-solid-state architecture is a sodium solid electrolyte that exhibits high Na+ conductivity at ambient temperatures, as well as excellent phase and electrochemical stability. In this work, we present the synthesis of a novel Cl-doped tetragonal Na 3PS4 (t-Na3−xPS4−xCl x) solid electrolyte with a room-temperature Na+ conductivity exceeding 1 mS cm−1. We demonstrate that an all-solid-state TiS2/ t-Na3−xPS4−xClx/Na cell utilizing this solid electrolyte can be cycled at room-temperature at a rate of C/10 with a capacity of over 100 mAh g−1 over 10 cycles. Finally, we provide experimental evidence that this excellent electrochemical performance is not only due to the high Na+ conductivity of the solid electrolyte, but also due to the effect that "salting" Na3PS4 has on the formation of an electronically insulating, ionically conducting solid electrolyte interphase.
546 $a English
590 $a School code: 0033
650 4 $a Nanoscience. $3 587832
650 4 $a Nanotechnology. $3 526235
650 4 $a Energy. $3 876794
650 4 $a Materials science. $3 543314
653 $a Battery
653 $a Electrochemistry
653 $a Electrolyte
653 $a Interphase
653 $a Solid state
653 $a Sulfide-based solid electrolytes
653 $a Superionic
690 $a 0565
690 $a 0652
690 $a 0791
690 $a 0794
710 2 $a University of California, San Diego. $b NanoEngineering. $e degree granting institution. $3 3816038
720 1 $a Meng, Ying Shirley $e degree supervisor.
773 0 $t Masters Abstracts International $g 78-11.
790 $a 0033
791 $a M.S.
792 $a 2017
856 4 0 $u https://pqdd.sinica.edu.tw/twdaoapp/servlet/advanced?query=10260155