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Reaction Pathways and Kinetics of Re...

Yu, Peng.

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Reaction Pathways and Kinetics of Reaction Coupling for Process Intensification.

紀錄類型:	書目-電子資源 : Monograph/item
正題名/作者:	Reaction Pathways and Kinetics of Reaction Coupling for Process Intensification./
作者:	Yu, Peng.
出版者:	Ann Arbor : ProQuest Dissertations & Theses, : 2021,
面頁冊數:	142 p.
附註:	Source: Dissertations Abstracts International, Volume: 82-12, Section: B.
Contained By:	Dissertations Abstracts International82-12B.
標題:	Chemical engineering. -
電子資源:	https://pqdd.sinica.edu.tw/twdaoapp/servlet/advanced?query=28418907
ISBN:	9798505599914

Reaction Pathways and Kinetics of Reaction Coupling for Process Intensification.
Yu, Peng.

Reaction Pathways and Kinetics of Reaction Coupling for Process Intensification. - Ann Arbor : ProQuest Dissertations & Theses, 2021 - 142 p.

Source: Dissertations Abstracts International, Volume: 82-12, Section: B.

Thesis (D.Eng.)--University of Massachusetts Lowell, 2021.

This item must not be sold to any third party vendors.

To improve process efficiency and safety and simultaneously reduce environmental pollution and operation cost, the concept of process intensification has gained increased attention. Process intensification seeks to develop new strategies of integrating multiple processes into one with a smaller footprint or optimizing an existing process for higher throughput. In this dissertation, process intensification is investigated by coupling two complementary reactions. The first system investigated is the coupling of ethylbenzene dehydrogenation and nitrobenzene hydrogenation over MoO3 based catalysts The reaction coupling concept is then extended into the emerging field of shale gas utilization, where four more reaction coupling schemes have been further investigated: (1) coupling propane pyrolysis with a radical generating reaction (i.e., nitrobenzene pyrolysis to generate phenyl radicals); (2) catalytic reaction coupling of propane dehydrogenation and nitrobenzene hydrogenation over Pt/Al2O3 catalysts; (3) coupling of propane dehydrogenation and hydrogenation of biomass-derived cresol over bifunctional catalysts, and (4) oxidative dehydrogenation of propane facilitated by NOx. For each study, the reaction pathways and chemical kinetics are elucidated to obtain a fundamental understanding of the reaction system. Such knowledge will serve as the foundation of applying the reaction coupling concept to the development of intensified process in the future.

ISBN: 9798505599914Subjects--Topical Terms:

560457
Chemical engineering.
Subjects--Index Terms:

Kinetic modeling

Reaction Pathways and Kinetics of Reaction Coupling for Process Intensification.
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500 $a Source: Dissertations Abstracts International, Volume: 82-12, Section: B.
500 $a Advisor: Wong, Hsi-wu.
502 $a Thesis (D.Eng.)--University of Massachusetts Lowell, 2021.
506 $a This item must not be sold to any third party vendors.
520 $a To improve process efficiency and safety and simultaneously reduce environmental pollution and operation cost, the concept of process intensification has gained increased attention. Process intensification seeks to develop new strategies of integrating multiple processes into one with a smaller footprint or optimizing an existing process for higher throughput. In this dissertation, process intensification is investigated by coupling two complementary reactions. The first system investigated is the coupling of ethylbenzene dehydrogenation and nitrobenzene hydrogenation over MoO3 based catalysts The reaction coupling concept is then extended into the emerging field of shale gas utilization, where four more reaction coupling schemes have been further investigated: (1) coupling propane pyrolysis with a radical generating reaction (i.e., nitrobenzene pyrolysis to generate phenyl radicals); (2) catalytic reaction coupling of propane dehydrogenation and nitrobenzene hydrogenation over Pt/Al2O3 catalysts; (3) coupling of propane dehydrogenation and hydrogenation of biomass-derived cresol over bifunctional catalysts, and (4) oxidative dehydrogenation of propane facilitated by NOx. For each study, the reaction pathways and chemical kinetics are elucidated to obtain a fundamental understanding of the reaction system. Such knowledge will serve as the foundation of applying the reaction coupling concept to the development of intensified process in the future.
590 $a School code: 0111.
650 4 $a Chemical engineering. $3 560457
653 $a Kinetic modeling
653 $a Process intensification
653 $a Propane
653 $a Reaction coupling
653 $a Shale gas
690 $a 0542
710 2 $a University of Massachusetts Lowell. $b Chemical Engineering. $3 3547571
773 0 $t Dissertations Abstracts International $g 82-12B.
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793 $a English
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