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Design and Application of Sustainabl...

Ye, Tao.

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Design and Application of Sustainable Pd-based Catalysts for Nitrite and Nitrate Reduction.

Record Type:	Electronic resources : Monograph/item
Title/Author:	Design and Application of Sustainable Pd-based Catalysts for Nitrite and Nitrate Reduction./
Author:	Ye, Tao.
Published:	Ann Arbor : ProQuest Dissertations & Theses, : 2018,
Description:	179 p.
Notes:	Source: Dissertations Abstracts International, Volume: 79-12, Section: B.
Contained By:	Dissertations Abstracts International79-12B.
Subject:	Environmental engineering. -
Online resource:	http://pqdd.sinica.edu.tw/twdaoapp/servlet/advanced?query=10824954
ISBN:	9780438010796

Design and Application of Sustainable Pd-based Catalysts for Nitrite and Nitrate Reduction.
Ye, Tao.

Design and Application of Sustainable Pd-based Catalysts for Nitrite and Nitrate Reduction. - Ann Arbor : ProQuest Dissertations & Theses, 2018 - 179 p.

Source: Dissertations Abstracts International, Volume: 79-12, Section: B.

Thesis (Ph.D.)--The George Washington University, 2018.

This item must not be sold to any third party vendors.

This dissertation focused on the development of sustainable Pd-based catalysts for the removal of waterborne contaminants (i.e., nitrite and nitrate). It explored different catalyst supports, including electrospun polyacrylonitrile (PAN) nanofibers (NFs), electrospun carbon nanofibers (CNFs), and graphitic carbon nitride (g-C3N4), which were underexplored for environmental engineering applications. Catalytic kinetics, selectivity (ammonia vs. nitrogen), and longevity for contaminant reduction were evaluated. Extensive instrumental analyses (e.g., scanning electron microscopy (SEM), transmission electron microscopy (TEM), and X-ray photoelectron spectroscopy (XPS)) were also conducted to identify key catalyst properties that determine catalytic performance. These Pd-based catalysts are effective, robust, and sustainable, and therefore they hold promise for water decontamination. The following topics were included in this dissertation: (1) Electrospun PAN Nanofiber Supported Pd Catalyst Composites for Water Decontamination; (2) Enhancement of Nitrite Reduction Kinetics on Electrospun Pd-Carbon Nanomaterial Catalysts for Water Purification; (3) g-C3N4 Supported Ultrafine Pd and Pd-Cu Catalysts: Enhanced Reactivity, Selectivity, and Longevity for Nitrite and Nitrate Hydrogenation.

ISBN: 9780438010796Subjects--Topical Terms:

548583
Environmental engineering.

Design and Application of Sustainable Pd-based Catalysts for Nitrite and Nitrate Reduction.
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520 $a This dissertation focused on the development of sustainable Pd-based catalysts for the removal of waterborne contaminants (i.e., nitrite and nitrate). It explored different catalyst supports, including electrospun polyacrylonitrile (PAN) nanofibers (NFs), electrospun carbon nanofibers (CNFs), and graphitic carbon nitride (g-C3N4), which were underexplored for environmental engineering applications. Catalytic kinetics, selectivity (ammonia vs. nitrogen), and longevity for contaminant reduction were evaluated. Extensive instrumental analyses (e.g., scanning electron microscopy (SEM), transmission electron microscopy (TEM), and X-ray photoelectron spectroscopy (XPS)) were also conducted to identify key catalyst properties that determine catalytic performance. These Pd-based catalysts are effective, robust, and sustainable, and therefore they hold promise for water decontamination. The following topics were included in this dissertation: (1) Electrospun PAN Nanofiber Supported Pd Catalyst Composites for Water Decontamination; (2) Enhancement of Nitrite Reduction Kinetics on Electrospun Pd-Carbon Nanomaterial Catalysts for Water Purification; (3) g-C3N4 Supported Ultrafine Pd and Pd-Cu Catalysts: Enhanced Reactivity, Selectivity, and Longevity for Nitrite and Nitrate Hydrogenation.
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