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Probing Transition Metal Dichalcogen...

Hill, Heather M.

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Probing Transition Metal Dichalcogenide Monolayers and Heterostructures by Optical Spectroscopy and Scanning Tunneling Spectroscopy.

Record Type:	Electronic resources : Monograph/item
Title/Author:	Probing Transition Metal Dichalcogenide Monolayers and Heterostructures by Optical Spectroscopy and Scanning Tunneling Spectroscopy./
Author:	Hill, Heather M.
Description:	136 p.
Notes:	Source: Dissertation Abstracts International, Volume: 77-08(E), Section: B.
Contained By:	Dissertation Abstracts International77-08B(E).
Subject:	Optics. -
Online resource:	http://pqdd.sinica.edu.tw/twdaoapp/servlet/advanced?query=10096878
ISBN:	9781339609652

Probing Transition Metal Dichalcogenide Monolayers and Heterostructures by Optical Spectroscopy and Scanning Tunneling Spectroscopy.
Hill, Heather M.

Probing Transition Metal Dichalcogenide Monolayers and Heterostructures by Optical Spectroscopy and Scanning Tunneling Spectroscopy. - 136 p.

Source: Dissertation Abstracts International, Volume: 77-08(E), Section: B.

Thesis (Ph.D.)--Columbia University, 2016.

Atomically thin two-dimensional materials, such as graphene and semiconductor transition metal dichalcogenides (TMDCs), exhibit remarkable and desirable optical and electronic properties. This dissertation focuses on the excitonic properties of monolayer TMDCs taken first in isolation and then in contact with another material.

ISBN: 9781339609652Subjects--Topical Terms:

517925
Optics.

Probing Transition Metal Dichalcogenide Monolayers and Heterostructures by Optical Spectroscopy and Scanning Tunneling Spectroscopy.
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020 $a 9781339609652
035 $a (MiAaPQ)AAI10096878
035 $a AAI10096878
040 $a MiAaPQ $c MiAaPQ
100 1 $a Hill, Heather M. $3 3192709
245 1 0 $a Probing Transition Metal Dichalcogenide Monolayers and Heterostructures by Optical Spectroscopy and Scanning Tunneling Spectroscopy.
300 $a 136 p.
500 $a Source: Dissertation Abstracts International, Volume: 77-08(E), Section: B.
500 $a Adviser: Tony F. Heinz.
502 $a Thesis (Ph.D.)--Columbia University, 2016.
520 $a Atomically thin two-dimensional materials, such as graphene and semiconductor transition metal dichalcogenides (TMDCs), exhibit remarkable and desirable optical and electronic properties. This dissertation focuses on the excitonic properties of monolayer TMDCs taken first in isolation and then in contact with another material.
520 $a We begin with a study of the exciton binding energy in two monolayer TMDCs, WS2 and MoS2. We observe excited states of the exciton by two dierent optical spectroscopy techniques: reflectance contrast and photoluminescence excitation (PLE) spectroscopy. We fit a hydrogenic model to the energies associated with the excited states and infer a binding energy, which is an order of magnitude higher than the bulk material.
520 $a In the second half of this work, we study two types of two-dimensional vertical heterostructures. First, we investigate heterostructures composed of monolayer WS2 partially capped with graphene one to four layers thick. Using reflectance contrast to measure the spectral broadening of the excitonic features, we measure the decrease in the coherence lifetime of the exciton in WS2 due to charge and energy transfer when in contact with graphene. We then compare our results with the exciton lifetime in MoS 2/WS2 and MoSe2/WSe2 heterostructures. In TMDC/TMDC heterostructures, the decrease in exciton lifetime is twice that in WS2/graphene heterostructures and due predominantly to charge transfer between the layers.
520 $a Finally, we probe the band alignment in MoS2/WS2 heterostructures using scanning tunneling microscopy (STM) and spectroscopy (STS). We confirm the monolayer band gaps and the predicted type II band alignment in the heterostructure. Drawing from all the research presented, we arrive at a favorable conclusion about the viability of TMDC based devices.
590 $a School code: 0054.
650 4 $a Optics. $3 517925
650 4 $a Theoretical physics. $3 2144760
650 4 $a Nanotechnology. $3 526235
690 $a 0752
690 $a 0753
690 $a 0652
710 2 $a Columbia University. $b Physics. $3 2101563
773 0 $t Dissertation Abstracts International $g 77-08B(E).
790 $a 0054
791 $a Ph.D.
792 $a 2016
793 $a English
856 4 0 $u http://pqdd.sinica.edu.tw/twdaoapp/servlet/advanced?query=10096878