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Semivolatile Organic Compounds in Sn...

McDaniel, Mark R.

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Semivolatile Organic Compounds in Snowmobile Emissions and in the Snowpack and Surface Water in Blackwood Canyon, Lake Tahoe, CA.

Record Type:	Language materials, printed : Monograph/item
Title/Author:	Semivolatile Organic Compounds in Snowmobile Emissions and in the Snowpack and Surface Water in Blackwood Canyon, Lake Tahoe, CA./
Author:	McDaniel, Mark R.
Description:	136 p.
Notes:	Source: Dissertation Abstracts International, Volume: 74-10(E), Section: B.
Contained By:	Dissertation Abstracts International74-10B(E).
Subject:	Environmental Sciences. -
Online resource:	http://pqdd.sinica.edu.tw/twdaoapp/servlet/advanced?query=3566275
ISBN:	9781303172380

Semivolatile Organic Compounds in Snowmobile Emissions and in the Snowpack and Surface Water in Blackwood Canyon, Lake Tahoe, CA.
McDaniel, Mark R.

Semivolatile Organic Compounds in Snowmobile Emissions and in the Snowpack and Surface Water in Blackwood Canyon, Lake Tahoe, CA. - 136 p.

Source: Dissertation Abstracts International, Volume: 74-10(E), Section: B.

Thesis (Ph.D.)--University of Nevada, Reno, 2013.

Snowpack in alpine environments contains appreciable levels of regional pollution acquired through natural processes of wet and dry deposition, as well as from immediate sources such as snowmobile engine exhaust. Understanding the fate and transport of those pollutants in alpine environments is a crucial step towards managing emission sources in alpine terrain to mitigate their impacts on natural resources. This study presents results from detailed chemical analysis for 168 species of semivolatile organic compounds (SVOC) in exhaust from snowmobile engines and in 58 samples of snow and surface water collected in Blackwood Canyon, a tributary to the west shore of Lake Tahoe and a popular winter recreation area for snowmobile riders. Snow and water samples were collected during a six week period in the spring of 2006. SVOC analyses included highly toxic and persistent polycyclic aromatic hydrocarbons (PAH), fossil fuel biomarker compounds hopanes and steranes, and saturated alkanes commonly found in fossil fuels, all of which are emitted as products of incomplete combustion and useful for identifying fossil fuel combustion emissions in the environment.

ISBN: 9781303172380Subjects--Topical Terms:

676987
Environmental Sciences.

Semivolatile Organic Compounds in Snowmobile Emissions and in the Snowpack and Surface Water in Blackwood Canyon, Lake Tahoe, CA.
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245 1 0 $a Semivolatile Organic Compounds in Snowmobile Emissions and in the Snowpack and Surface Water in Blackwood Canyon, Lake Tahoe, CA.
300 $a 136 p.
500 $a Source: Dissertation Abstracts International, Volume: 74-10(E), Section: B.
500 $a Adviser: Barbara Zielinska.
502 $a Thesis (Ph.D.)--University of Nevada, Reno, 2013.
520 $a Snowpack in alpine environments contains appreciable levels of regional pollution acquired through natural processes of wet and dry deposition, as well as from immediate sources such as snowmobile engine exhaust. Understanding the fate and transport of those pollutants in alpine environments is a crucial step towards managing emission sources in alpine terrain to mitigate their impacts on natural resources. This study presents results from detailed chemical analysis for 168 species of semivolatile organic compounds (SVOC) in exhaust from snowmobile engines and in 58 samples of snow and surface water collected in Blackwood Canyon, a tributary to the west shore of Lake Tahoe and a popular winter recreation area for snowmobile riders. Snow and water samples were collected during a six week period in the spring of 2006. SVOC analyses included highly toxic and persistent polycyclic aromatic hydrocarbons (PAH), fossil fuel biomarker compounds hopanes and steranes, and saturated alkanes commonly found in fossil fuels, all of which are emitted as products of incomplete combustion and useful for identifying fossil fuel combustion emissions in the environment.
520 $a Average SVOC concentrations in background snow were as follows: total PAH was 200+/-12 ng.l-1, with 16+/-1.3 ng.l-1 PAH with three or more aromatic rings; hopanes and steranes were 56+/- 3 ng.l -1; and total alkanes were 9,900+/- 500 ng.l-1. Average background SVOC concentrations were used to estimate background SVOC surface loading (microg.m-2). Loadings in excess of the estimated background are mapped and compared with observations of snowmobile activity to determine effects of snowmobile emissions on snow water quality. Loading of PAH in snow was found to be significantly greater than background loading (alpha=5%) where snowmobile tracks cover more than 50% of the snow surface. Loadings were eight to 20 times greater than background levels where snowmobile traffic was heaviest over snow covered roads.
520 $a SVOC were also measured in snow melt and surface water samples in Blackwood Canyon for comparison with chemical profiles in snow samples. Flux of SVOC (g.day-1) from Blackwood Creek into Lake Tahoe was calculated and compared to estimates of background flux. Initially comparable to background estimates, PAH flux was found to have increased from background levels at 74 g.day-1 to 160 g.day-1 in four days. In another sample collected eight days after the initial sample, PAH flux had increased to 480 g.day-1. Cumulative impacts to Blackwood Creek and downstream to Lake Tahoe may be inferred from the discharge hydrograph, but should be further characterized with routine sampling through the entire snowmelt period.
590 $a School code: 0139.
650 4 $a Environmental Sciences. $3 676987
650 4 $a Chemistry, Analytical. $3 586156
690 $a 0768
690 $a 0486
710 2 $a University of Nevada, Reno. $b Atmospheric Sciences. $3 1019574
773 0 $t Dissertation Abstracts International $g 74-10B(E).
790 $a 0139
791 $a Ph.D.
792 $a 2013
793 $a English
856 4 0 $u http://pqdd.sinica.edu.tw/twdaoapp/servlet/advanced?query=3566275