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Optical Kerr effect spectroscopy usi...

Zhu, Xiang.

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Optical Kerr effect spectroscopy using dual-pulse-excitation scheme.

紀錄類型:	書目-電子資源 : Monograph/item
正題名/作者:	Optical Kerr effect spectroscopy using dual-pulse-excitation scheme./
作者:	Zhu, Xiang.
面頁冊數:	62 p.
附註:	Source: Masters Abstracts International, Volume: 43-06, page: 2233.
Contained By:	Masters Abstracts International43-06.
標題:	Chemistry, Analytical. -
電子資源:	http://pqdd.sinica.edu.tw/twdaoapp/servlet/advanced?query=1431048
ISBN:	0542035138

Optical Kerr effect spectroscopy using dual-pulse-excitation scheme.
Zhu, Xiang.

Optical Kerr effect spectroscopy using dual-pulse-excitation scheme. - 62 p.

Source: Masters Abstracts International, Volume: 43-06, page: 2233.

Thesis (M.S.)--Boston College, 2005.

Optical Kerr effect (OKE) spectroscopy has found broad use in monitoring ultrafast dynamics in transparent media. Interest is also developing in using OKE spectroscopy as a means of achieving contrast in nonlinear microscopy. I demonstrated that by using two pump pulses with independently-controllable polarizations, intensity and timing, different contributions to the OKE signal in liquids can be enhanced and suppressed. Then I characterize in detail the perpendicularly-polarized pulses used for the excitation step in OKE spectroscopy. The results indicate that the signal can be described well as arising from the sum of independent third-order responses initiated by each pump pulses. These experiments pave the way for using sequences of multiple pump pulses to single out the contribution of a single mode of interest. Such a technique would be of interest for performing mode-selective OKE microscopy.

ISBN: 0542035138Subjects--Topical Terms:

586156
Chemistry, Analytical.

Optical Kerr effect spectroscopy using dual-pulse-excitation scheme.
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502 $a Thesis (M.S.)--Boston College, 2005.
520 $a Optical Kerr effect (OKE) spectroscopy has found broad use in monitoring ultrafast dynamics in transparent media. Interest is also developing in using OKE spectroscopy as a means of achieving contrast in nonlinear microscopy. I demonstrated that by using two pump pulses with independently-controllable polarizations, intensity and timing, different contributions to the OKE signal in liquids can be enhanced and suppressed. Then I characterize in detail the perpendicularly-polarized pulses used for the excitation step in OKE spectroscopy. The results indicate that the signal can be described well as arising from the sum of independent third-order responses initiated by each pump pulses. These experiments pave the way for using sequences of multiple pump pulses to single out the contribution of a single mode of interest. Such a technique would be of interest for performing mode-selective OKE microscopy.
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