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Optical Kerr effect spectroscopy usi...
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Zhu, Xiang.
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Optical Kerr effect spectroscopy using dual-pulse-excitation scheme.
Record Type:
Electronic resources : Monograph/item
Title/Author:
Optical Kerr effect spectroscopy using dual-pulse-excitation scheme./
Author:
Zhu, Xiang.
Description:
62 p.
Notes:
Source: Masters Abstracts International, Volume: 43-06, page: 2233.
Contained By:
Masters Abstracts International43-06.
Subject:
Chemistry, Analytical. -
Online resource:
http://pqdd.sinica.edu.tw/twdaoapp/servlet/advanced?query=1431048
ISBN:
0542035138
Optical Kerr effect spectroscopy using dual-pulse-excitation scheme.
Zhu, Xiang.
Optical Kerr effect spectroscopy using dual-pulse-excitation scheme.
- 62 p.
Source: Masters Abstracts International, Volume: 43-06, page: 2233.
Thesis (M.S.)--Boston College, 2005.
Optical Kerr effect (OKE) spectroscopy has found broad use in monitoring ultrafast dynamics in transparent media. Interest is also developing in using OKE spectroscopy as a means of achieving contrast in nonlinear microscopy. I demonstrated that by using two pump pulses with independently-controllable polarizations, intensity and timing, different contributions to the OKE signal in liquids can be enhanced and suppressed. Then I characterize in detail the perpendicularly-polarized pulses used for the excitation step in OKE spectroscopy. The results indicate that the signal can be described well as arising from the sum of independent third-order responses initiated by each pump pulses. These experiments pave the way for using sequences of multiple pump pulses to single out the contribution of a single mode of interest. Such a technique would be of interest for performing mode-selective OKE microscopy.
ISBN: 0542035138Subjects--Topical Terms:
586156
Chemistry, Analytical.
Optical Kerr effect spectroscopy using dual-pulse-excitation scheme.
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Optical Kerr effect (OKE) spectroscopy has found broad use in monitoring ultrafast dynamics in transparent media. Interest is also developing in using OKE spectroscopy as a means of achieving contrast in nonlinear microscopy. I demonstrated that by using two pump pulses with independently-controllable polarizations, intensity and timing, different contributions to the OKE signal in liquids can be enhanced and suppressed. Then I characterize in detail the perpendicularly-polarized pulses used for the excitation step in OKE spectroscopy. The results indicate that the signal can be described well as arising from the sum of independent third-order responses initiated by each pump pulses. These experiments pave the way for using sequences of multiple pump pulses to single out the contribution of a single mode of interest. Such a technique would be of interest for performing mode-selective OKE microscopy.
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http://pqdd.sinica.edu.tw/twdaoapp/servlet/advanced?query=1431048
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