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Investigation of Sulfide-based Solid...

Kompella, Christopher,

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Investigation of Sulfide-based Solid Electrolytes for Sodium All-Solid-State Rechargeable Batteries /

紀錄類型:	書目-電子資源 : Monograph/item
正題名/作者:	Investigation of Sulfide-based Solid Electrolytes for Sodium All-Solid-State Rechargeable Batteries // Christopher Kompella.
作者:	Kompella, Christopher,
面頁冊數:	1 electronic resource (63 pages)
附註:	Source: Masters Abstracts International, Volume: 78-11.
Contained By:	Masters Abstracts International78-11.
標題:	Nanoscience. -
電子資源:	https://pqdd.sinica.edu.tw/twdaoapp/servlet/advanced?query=10260155
ISBN:	9781369696837

Investigation of Sulfide-based Solid Electrolytes for Sodium All-Solid-State Rechargeable Batteries /
Kompella, Christopher,

Investigation of Sulfide-based Solid Electrolytes for Sodium All-Solid-State Rechargeable Batteries /Christopher Kompella. - 1 electronic resource (63 pages)

Source: Masters Abstracts International, Volume: 78-11.

All-solid-state sodium-ion batteries are promising candidates for large-scale energy storage applications. The key enabler for an all-solid-state architecture is a sodium solid electrolyte that exhibits high Na+ conductivity at ambient temperatures, as well as excellent phase and electrochemical stability. In this work, we present the synthesis of a novel Cl-doped tetragonal Na 3PS4 (t-Na3−xPS4−xCl x) solid electrolyte with a room-temperature Na+ conductivity exceeding 1 mS cm−1. We demonstrate that an all-solid-state TiS2/ t-Na3−xPS4−xClx/Na cell utilizing this solid electrolyte can be cycled at room-temperature at a rate of C/10 with a capacity of over 100 mAh g−1 over 10 cycles. Finally, we provide experimental evidence that this excellent electrochemical performance is not only due to the high Na+ conductivity of the solid electrolyte, but also due to the effect that "salting" Na3PS4 has on the formation of an electronically insulating, ionically conducting solid electrolyte interphase.

English

ISBN: 9781369696837Subjects--Topical Terms:

587832
Nanoscience.
Subjects--Index Terms:

Battery

Investigation of Sulfide-based Solid Electrolytes for Sodium All-Solid-State Rechargeable Batteries /
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502 $b M.S. $c University of California, San Diego $d 2017.
520 $a All-solid-state sodium-ion batteries are promising candidates for large-scale energy storage applications. The key enabler for an all-solid-state architecture is a sodium solid electrolyte that exhibits high Na+ conductivity at ambient temperatures, as well as excellent phase and electrochemical stability. In this work, we present the synthesis of a novel Cl-doped tetragonal Na 3PS4 (t-Na3−xPS4−xCl x) solid electrolyte with a room-temperature Na+ conductivity exceeding 1 mS cm−1. We demonstrate that an all-solid-state TiS2/ t-Na3−xPS4−xClx/Na cell utilizing this solid electrolyte can be cycled at room-temperature at a rate of C/10 with a capacity of over 100 mAh g−1 over 10 cycles. Finally, we provide experimental evidence that this excellent electrochemical performance is not only due to the high Na+ conductivity of the solid electrolyte, but also due to the effect that "salting" Na3PS4 has on the formation of an electronically insulating, ionically conducting solid electrolyte interphase.
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653 $a Sulfide-based solid electrolytes
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