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Developing Advanced Materials for Ca...

Esmaeilirad, Mohammadreza.

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Developing Advanced Materials for Carbon Dioxide Electroreduction to Value-added Chemicals and Fuels.

Record Type:	Electronic resources : Monograph/item
Title/Author:	Developing Advanced Materials for Carbon Dioxide Electroreduction to Value-added Chemicals and Fuels./
Author:	Esmaeilirad, Mohammadreza.
Published:	Ann Arbor : ProQuest Dissertations & Theses, : 2023,
Description:	186 p.
Notes:	Source: Dissertations Abstracts International, Volume: 85-03, Section: B.
Contained By:	Dissertations Abstracts International85-03B.
Subject:	Chemical engineering. -
Online resource:	https://pqdd.sinica.edu.tw/twdaoapp/servlet/advanced?query=30575844
ISBN:	9798380166195

Developing Advanced Materials for Carbon Dioxide Electroreduction to Value-added Chemicals and Fuels.
Esmaeilirad, Mohammadreza.

Developing Advanced Materials for Carbon Dioxide Electroreduction to Value-added Chemicals and Fuels. - Ann Arbor : ProQuest Dissertations & Theses, 2023 - 186 p.

Source: Dissertations Abstracts International, Volume: 85-03, Section: B.

Thesis (Ph.D.)--Illinois Institute of Technology, 2023.

Developing highly efficient electrocatalysts for the carbon dioxide reduction reaction (CO2RR) to value-added fuels and chemicals offers a feasible pathway for renewable energy storage and could help mitigate the ever-increasing carbon dioxide (CO2) emissions from human activities. Different catalysts are known to catalyze CO2RR in aqueous solutions. Most known catalysts are only capable of transferring 2 electrons with needed protons to CO2 producing either carbon monoxide (CO) or formic acid (HCOOH). Copper (Cu) is the only electrocatalytic material that converts CO2 into different types of hydrocarbon products. Additionally, owing to Cu's natural abundance and low cost, it has been intensively studied for CO2RR for decades. However, the required high input energy (overpotential), low product selectivity towards valuable fuel products and the lack of long-term stability remain major challenges for Cu-based catalysts. This work aims to develop new materials that produce hydrocarbons at lower overpotentials with higher rates and greater selectivity than current copper catalysts. By implementing a process referred to as the electrocatalyst discovery cycle iterations between predications, catalyst testing, and active site characterization allow for the rational design and discovery of new and improved electrocatalysts for CO2RR. This methodology led to the discovery of different heteroatomic catalysts as low overpotential catalysts for electroreduction of CO2 high energy density hydrocarbon products.

ISBN: 9798380166195Subjects--Topical Terms:

560457
Chemical engineering.
Subjects--Index Terms:

Electrochemical engineering

Developing Advanced Materials for Carbon Dioxide Electroreduction to Value-added Chemicals and Fuels.
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520 $a Developing highly efficient electrocatalysts for the carbon dioxide reduction reaction (CO2RR) to value-added fuels and chemicals offers a feasible pathway for renewable energy storage and could help mitigate the ever-increasing carbon dioxide (CO2) emissions from human activities. Different catalysts are known to catalyze CO2RR in aqueous solutions. Most known catalysts are only capable of transferring 2 electrons with needed protons to CO2 producing either carbon monoxide (CO) or formic acid (HCOOH). Copper (Cu) is the only electrocatalytic material that converts CO2 into different types of hydrocarbon products. Additionally, owing to Cu's natural abundance and low cost, it has been intensively studied for CO2RR for decades. However, the required high input energy (overpotential), low product selectivity towards valuable fuel products and the lack of long-term stability remain major challenges for Cu-based catalysts. This work aims to develop new materials that produce hydrocarbons at lower overpotentials with higher rates and greater selectivity than current copper catalysts. By implementing a process referred to as the electrocatalyst discovery cycle iterations between predications, catalyst testing, and active site characterization allow for the rational design and discovery of new and improved electrocatalysts for CO2RR. This methodology led to the discovery of different heteroatomic catalysts as low overpotential catalysts for electroreduction of CO2 high energy density hydrocarbon products.
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